Добавил:
Опубликованный материал нарушает ваши авторские права? Сообщите нам.
Вуз: Предмет: Файл:

brechignac_f_desmet_g_eds_equidosimetry_ecological_standardi

.pdf
Скачиваний:
2
Добавлен:
19.11.2019
Размер:
5.12 Mб
Скачать

358

The whole Ukrainian contingent of peace-making forces participated in the observance of safety at performing their tasks in districts where weapons with depleted uranium were used.

Inspection of cars has revealed the presence Cs-137. The maximal pollution made 482.3 Bq/m2. It is below minimally allowable activity on workplaces under requirements of the Ukrainian standards. With all divisions deactivation of the engineering gear was carried out. All cars were deactivated.

Inspection of places of aviation impacts in the zone under the responsibility of the Ukrainian peace-making contingent and in places of performance of tasks has revealed pollution radionuclides Cs-137, Th-232 and Ra-226.

The basic conclusions of the carried out work were:

ξ

threats to the Ukrainian peace-making contingent it is not revealed;

ξ

the zone of a disposition of the Ukrainian peace-making contingent has no

 

territories polluted with the depleted uranium;

ξ

the decision on creation of a uniform complex of the equipment for radiation

 

monitoring and the control was correct;

ξ

VECTOR, SKRINER and DMC 2000 complexes have confirmed high

 

efficiency;

ξ

the obtained experience allows improving of radiating safety system.

6. Conclusions

The overall objective of sanitary-and-hygienic normalization is studying and substantiation of limits of intensity and duration of actions on people in conditions of impact of harmful substances [9, 12].

359

The considered types of military activity confirm an urgency of application of methods of sanitary-and-hygienic normalization with the purpose:

ξ

choice of parameters on which the establishment of the fact of occurrence of a

 

new source of pollution is possible;

ξ

studying and substantiation of the boundary values, the chosen parameters

 

which authentically confirm presence of pollution.

References

1.The Law of Ukraine about the protection of the population and territory from the extreme situations of technogenic and natural character (in Ukrainian)

2.The Law of Ukraine about the area of extreme ecological situation (in Ukrainian)

3.Decree of the Parliament of Ukraine about the main directions of the government policy of Ukraine in the branch of the environmental protection, use of natural resources and securing of ecological safety, 05.03.98 ʋ 188/98-BP (in Ukrainian)

4.Decree of the Parliament of Ukraine about the conception of the state regulation of the safety and management of nuclear branch of Ukraine, 25.01.94 ʋ 3871-XII (in Ukrainian)

5.Decree of the Cabinet of Ministers of Ukraine about the approval Composite programme the radioactive wastes treatment of 29.04.96 ʋ 480 (with changes, made by Decree of the Cabinet of Ministers of Ukraine 05.04.99 ʋ 542 (in Ukrainian)

6.Decree of the President of Ukraine 23.02.2000 about the primary measures of the implementation of the Message of the President of Ukraine to the Parliament of Ukraine "Ukraine, entrance into XXI century. Strategy of economic and social development for 2000-2004" (in Ukrainian)

7.Charter about the particular partnership between Ukraine and Organisation of the North Atlantic Treaty, 09.07.97, Madrid (Spain) (in Ukrainian)

8.Yu. Izrael. Ecology and control of environment. Leningrad, Hydrometeoizdat, 1984 (in Russian)

9.A. Kachinsky. Risk concept in the context of ecological security of Ukraine. National institute of strategic research. Vol. 14, Kyiv, 1993 (in Ukrainian)

10.A. Kachinsky. Modern problems of ecological security of Ukraine. National institute of strategic research. Vol. 33, Kyiv, 1994 (in Ukrainian)

11.A. Kachinsky,O. Lavrinenko. War in Yugoslavia as a technogenic ecological catastrophe. Strategichna Panorama, Vol. 1-2, 2000 (in Ukrainian)

12.A. Kachinsky, O. Nakonechny. Stability of ecosystems and problem of standardization in the ecological security of Ukraine. National institute of strategic research. Series “Ecological security”, Vol. 1, Kyiv, 1996 (in Ukrainian)

13.A. Kachinsky, G.Khmil’. Ecological security of Ukraine: analysis, estimation and state policy. National institute of strategic research. Series “Ecological security”, Vol. 3, Kyiv, 1997 (in Ukrainian)

14.S.Zgourets. Start-1, or steeplechase. Narodna Armiya, 23.12.1999 (in Ukrainian)

15.V. Kovalevsky. Concept of evaluation ecological stay the military sites. Proceedings. Defence technologies, Vol.1, Kyiv 1998 (in Ukrainian)

16.V. Litovkin. Second Chernobyl matures at the missile shafts (?) of Ukraine. Izvestia, 16.2.1993 (in Russian)

17.O. Saltykov. Ecological standardization. Problems and perspectives. Ecologia, - 1989, #3 (in Russian)

18.The State programme of the Ukrainian Armed Forces reform and development until 200

19.V. Kovalevskyi, Radiological control and monitoring on the military installation sites in Ukraine. General approaches, SCOPE-RADSITE 12-14.11.98, “Radioactivity from Military Installation sites and Effects on Population Health”, Brussels, Belgium

20.E. Prohach. The ecology of nuclear disarmament. (scientific report). The World of Security VIII, International Institute on Global and Regional Security, Kyiv, 1995

LANDSCAPE CRITICALITY INDEXES FOR THE DIFFERENT POLLUTANTS

N. GRYTSYUK

Ukrainian Institute of Agricultural Radiology,

7, Mashynobudivnykiv St. Chabany, Kyiv prov. 255207 UKRAINE root@inrad..kiev.ua

V. DAVYDCHUK

Institute of Geography, National Academy of Sciences, 44 Volodymyrska St. 01034 Kyiv, UKRAINE chornob@geogr.freenet.kiev.ua

1. Introduction

Landscape can be defined as a multidimensional and multileveled spatial structure, which unites systematically such natural components as an earth crust with its lithology and relief, ground water, air, vegetation cower and animal population, as well as a soil, which is a result of their interaction. Landscape plays a role for an environment and can be characterized by a number of geochemical parameters, which reflect pathways, barriers, fluxes and balances of redistribution for the different substances, including pollutants. So both a primary and secondary contamination field is forming and evolving within the landscape, under influence of the landscape factors.

This permits use of the landscape approach for the monitoring of different pollutants and further evolution of the ecological situation, for the identification of the ecologically vulnerable landscapes.

Generally the landscape approach in ecotoxicology means a substantiation of the influence of the the sum of natural factors, which evolve themselves (relief, lithology, soil and vegetation cover, geochemical pathways and barriers), on the migration and accumulation of the pollutants, and identification of some areas, which are critical by the combination of these factors.

2. Landscape criticality factors

From this point of view, the criticality of landscape is a result of co-influence of the negative natural factors, which cause the pollutant accumulation at the geochemical barriers, or their intensive biogenic migration and accumulation by the biomass. As the landscape is positioned at the initial link of the trophic/food chain, its criticality reflects the potential risk of the pollutant bioavailability.

Because of chemical similarity of the number of technogenic pollutants (radionuclides and heavy metals etc.), the same methodological approach can be used in ecotoxicology. The ecotoxicological criticality of the landscapes can be defined via indexes of the pollutant balances for the elements of landscape structure and intensity of their biogenic migration.

361

F. Brechignac and G. Desmet (eds.), Equidosimetry, 361–368.

© 2005 Springer. Printed in the Netherlands.

362

3. Radiological criticality indexes

For the long-term evaluations and predictions of the pollutants behaviour, to considering the intensity of their horizontal migration and spontaneous decay are of special importance. The experimental data confirm very low velocity of the radionuclides re-distribution between landscape elements by the washing-off at the local level. The 137Cs and 90Sr annual transfer between geochemically adjacent landscapes is about 1% [3], which is less than their losses by physical decay. At least, it means: the consideration of the horizontal migration input/output in the mid-term evaluations is desirable. Moreover, this is essential for the long-living pollutants behaviour forecasting and migration ability evaluation.

The Chornobyl experience increasingly shows the migration processes intensity from the automorphous landscapes to the hydromorphous superaquatic ones, and this is in good correlation with the 137Cs transfer factor meanings for grass and wood [1, 4].

The balance of the radionuclides between different elements of the landscape structure, which are positioned at the different locations of the relief (plateau, slope, pediment or depression), reflects the ability of the ecosystem to evacuate or to collect the pollutants [3]. Both intensity and sign of the pollutant migration varies, following the combination of the landscape factors. Depending on the sign of the migration, the pollutant balance for an areal can be defined as:

ξ negative (green, predomination of the pollutant evacuation); ξ positive (orange, predomination of its accumulation);

ξ neutral (yellow), where processes of the evacuation and accumulation are balanced in equilibrium (Figure 1).

Fig. 1. 137Cs balances at the landscape areals of the Narodychi district.

363

Intensity of the migration varies in the different landscapes, and areals with a strong, intermediate or low evacuation/accumulation of the pollutants reflect the thin local variations of the soil forming deposit lithology, soil, and vegetation cover. Generally, most intensive redistribution of the radionuclides and other pollutants by surface migration are expected at the steep open slope surfaces, which connect autonomous and hydromorphic landscape areals. The mostly intensive accumulation is observed at the slope pediments and the bottoms of depressions, which reflects a role of mechanical geochemical barriers in the accumulation of the surface-migrating pollutants.

The approach used makes it possible to mapping the balance evaluations at the basis of a landscape map. Figure 1 shows intensity and balances of the redistribution of 137Cs or other corresponding pollutant by the washing-off/accumulation for the Narodychi district of Zhytomyr province at the qualitative level. Using appropriate experimental data, this can be transformed into quantitative evaluation, and such a quantitative balance index is one of the landscape criticality indexes.

The phytocoenoses as a biogeochemical barrier consume the pollutant movable forms from soil and ground water and disable that in the phytomass, more or less, depending of their radiological or ecotoxicological capacity and criticality. The transfer factor (TF) is an integral quantitative index, which reflects co-influence of the geochemical, geophysical, and biological factors on the intensity of the biogenic migration, and it can be used for the evaluation of the ecotoxicological criticality (Table 1 and Figure 2).

Fig. 2. Means of Tf 137Cs for the natural and cultivated grass associations (Narodychi district, agricultural lands withdrawn).

364

Table 1. Means of the 137Cs TF to the phytomass of the natural and cultivated grass at the different landscape areals

Means of TF,

Soils and landscape areals under

Soils and landscape areals under

Bqƒkg-

cultivated grass associations

natural grass associations

1/kBkƒm-2

 

 

0,1 - 0,2

Moraine-fluvioglacial plains and river

-

 

terraces with soddy-podzolic loamy

 

 

soils, covered by permanent grass

 

 

associations with predomination of

 

 

Dactylis glomerata L.

 

0,2 - 0,3

Moraine-fluvioglacial plains, river

Moraine-fluvioglacial plains and river

 

terraces and flood plains with soddy-

terraces with soddy-podzolic loamy

 

podzolic dusty-sandy and loamy gleic

soils, covered by meadows with

 

soils, covered by permanent grass

predomination of herbs and legumes

 

associations with predomination of

 

 

herbs

 

0,3 - 1,0

Moraine-fluvioglacial plains, river

Moraine-fluvioglacial plains, river

 

terraces, flood plains, and dells with

terraces and flood plains with soddy-

 

soddy-podzolic and soddy dusty-

podzolic dusty-sandy and loamy gleic

 

sandy and loamy gleyic soils, covered

soils, covered by the meadows with

 

by the permanent grass (herb)

predomination of xerophytous herbs

 

associations

 

1,0 - 3,0

Lowered moraine-fluvioglacial plains,

Moraine-fluvioglacial plains, river

 

river terraces and flood plains, dells

terraces and flood plains, and dells

 

and depressions with soddy-podzolic

with soddy-podzolic and soddy dusty-

 

sandy gley soils and silt bog soils,

sandy and loamy gleyic soils, alluvial

 

covered by permanent grass herb-

gleic loamy soils, covered by

 

legume associations

meadows with predomination of herb

 

 

and herb-legume associations

3,0 - 10,0

Lowered drained river terraces and

Moraine-fluvioglacial plains, river

 

flood plains with peat bog soils,

terraces and flood plains, and dells

 

covered by permanent grass herb-

with soddy-podzolic and soddy sandy

 

legume associations

gley soils and drained peaty soils,

 

 

covered by meadows with

 

 

predomination of herb and herb-

 

 

legume associations

10,0 - 20

-

Lowered drained river terraces and

 

 

flood plains with (alluvial) drained

 

 

peaty soils, covered by meadows with

 

 

predomination of grasses, herbs and

 

 

sedges

20,0 - 80...

-

Lowered drained river terraces and

 

 

flood plains with (alluvial) non-

 

 

drained peat bog soils, covered by

 

 

herb-sedgeous meadows

365

Results of studies of the 137Cs soil-plant transfer factor dependence upon landscape structure of the area show that such integral characteristic of biogenic radionuclide migration as TF correlates strongly with the landscape structure of the

territory. Consequent analysis and summarising of data allowed to obtaining the following table as an algorithm for the legend to TF map elaboration on the base of the

landscape approach.

4. Some evaluations and applications

Data presented in the Table 1 show, that the lowest criticality is specified for automorphous landscapes with low TF values, their meanings mount to 0,1-0,2 for sown grasses, and 0,2-0,3 for natural meadow coenoses. They were estimated for soddy-podzolic sandy loamy and loamy non-gleic soils of the river terraces and moraine-fluvioglacial plains. These soils of the Northern Ukrainian Woodland are characterised by the highest natural fertility and favourable water-physical properties. Moreover, these soils are typical for landscape areals occupying relatively raised, well drained locations with relatively good conditions of surface washing-off and additive potential of self-cleaning from radionuclides due to horizontal outflow during a longterm period. These areals as low critical ones with regard to radiological aspect could be considered as mostly attractive ones for the rehabilitation activity.

Average TF values equal to 0,2-1,0 for sown grasses and 0,3-3,0 for natural meadows are usual to soddy-podzolic sandy loam and loamy gleic soils, soddy-podzolic sandy soils gleic to different extent and alluvial soddy gleic loamy soils. This group includes soils significantly differed by the fertility and their position in landscape. The third group includes soils with highest values of TF, as peaty gleic, peat bog and alluvial peat bog soils. Transfer factor values in these soils mount to 3,0-10,0 for sown grasses and 10,0-80 for meadow coenosis. Alluvial soddy gleic sandy soils draw near to organogenic alluvial ones by high TF values. So, the highest level of radiological criticacy is characteristic for landscape areals in low located territories of hydromorphic type. Level of hydromorphism (automorphism) is determined not only by the type of soil, but also by the location in a relief, its hydrological regime, and the type of plant association. By whole natural properties these areals are considered to be little suitable for use even in conditions of low radioactive contamination.

Extent of soil cultivation influences significantly on 137Cs plant to soils transfer. At the same landscape conditions 137Cs TF for sown grasses on cultivated soils and in natural coenosis on non-cultivated ones can differ more than two orders of magnitude.

Data obtained show that the same radiological criticality level can be observed for landscape areals with types of soils and plant association sufficiently different, formed in various types of relief, but similar by the edaphic (grooving) conditions - fertility and humidity of soils. This fact shows, that the landscape influence due to completeness of natural factors is very important, hence it is very difficult to reveal the mostly important one. The last one concerns meadow coenoses especially, characterised by wide ecological amplitude.

The next step, predetermined by estimated regularity between TF and landscape structure of territory, became the cartographic interpretation of the factor values space distribution on the base of the landscape map. On the table data are

366

presented above the map of TF for the abandoned agricultural lands of Narodychi district (Figure 2).

The map characterizes, at the new level, patterns of the spatial distribution of the TF meanings for the natural and cultivated grass associations. It was used for solving a number of the radiological tasks, both scientific and practical, which are related to the factors of the biogenic migration of the radionuclides. Among them there are the evaluation and forecast of the potential contamination of the agricultural products for the abandoned lands of the Narodychi district, to support the decision making in the rehabilitation of these lands. By the overlay the TF map and 137Cs soil contamination map, the maps of potential 137Cs contamination for hay, and therefore maps for the milk and meat (Figures 3, 4, 5) were generated.

Being based on the actual experimental data, TF mean maps can be used correctly within at least nearest years, if hydro-termic (climatic) conditions are appropriate. For the further perspective, the map will be useful, if the actual TF meanings would be corrected at the base of the TF evolution forecast.

As the grass belongs to the easily contaminated phytomass fractions, the grass TF maps are very useful for the evaluations of the criticality the agricultural lands under any crops.

Fig. 3. Forecast of the natural and sowed grass hay by 137Cs contamination.

367

368

5. Conclusion

The effect of the landscape indication permits a reliable inter-component crossidentification within the landscape. Thus, the landscape approach to the evaluation the criticality indexes can be used for the radioecological evaluations, even if the

environmental characteristics of the territory affected are limited or non-reliable. The approach seems to be useful also in the general ecotoxicology, as the behaviour

characteristics of any pollutant of interest can be easily adopted.

6. References

1.Grytsyuk N. Dependence of Cs137 transfer factor for grass on the landscape structure of territory. Visnyk Agrarnych Nauk,. ¹ 4, 2001, p.97-99 (in Ukrainian)

2.Davydchuk V., Cs-137 balance in the Chornobyl exclusion zone. Ukrainian Geographic Journal, 1996, ¹1, p.39-44.

3.Davydchuk V., Zaroudna R. et al. Landscapes of Chernobyl zone and their estimation on the radionuclides migration conditions. Kiev, Naukova Dumka, 1994, 112 p. (in Russian).

4.Sorokina L. On accumulation of Cs137 by phytocomponents of forest ecosystems depending on edaphic conditions. Ukrainian Geographic Journal, 1996, ¹1, pp. 44-48(in Ukrainian)